Hot Brownian Colloids – talk

On 19th Jan 2023, I gave a ~40 min talk on “Hot Brownian Colloids in Structured Optical Tweezers” in a very interesting conference on Frontiers in Non-Equilibrium Physics (FNEP) held at Institute of Mathematical Sciences, Chennai.

I mainly spoke about emergent Brownian dynamics of laser-heated colloids under optical confinement. Below is the link to the talk.

I concluded my talk quoting P W Anderson’s essay “More is Different

“The constructionist hypothesis breaks down when confronted with the twin difficulties of scale and complexity.  The behavior of large and complex aggregates of elementary particles, it turns out, is not to be understood in terms of a simple extrapolation of the properties of a few particles.

Instead, at each level of complexity entirely new properties appear, and the understanding of the new behaviors requires research which I think is as fundamental in its nature as any other.”

P.W. Anderson  ‘More is Different’
Science, 177, 4047 (1972)

More is not only different, but also wonderful !

My talk at ICTS

On 1st Dec 2022, I gave a talk on “Structured-Light Scattering : Implications in Momentum Space” as part of a discussion meeting on STRUCTURED LIGHT AND SPIN-ORBIT PHOTONICS held at International Center of Theoretical Sciences, Bangalore.

I mainly spoke about topological light scattering in the frame work of angular momentum of light and absorptive effects in optothermal tweezers created by structured light.

Below is the embedded video link to my talk. The playlist also has many other interesting talks related to the topic.

Review article – Plasmonic colloids + Optical Vortex

Appended is a link to arxiv preprint of an invited review article that I wrote as part of a special issue on nanophotonics in the Indian Journal of Physics and Applied Physics. The issue is edited by Dr. Achanta Venugopal (TIFR/NPL).

In this review, I discuss about assembly and dynamics of plasmonic colloids under the influence of optical vortex fields.

The abstract reads :
Structured light has emerged as an important tool to interrogate and manipulate matter at micron and sub-micron scale. One form of structured light is an optical vortex beam. The helical wavefront of these vortices carry orbital angular momentum which can be transferred to a Brownian colloid. When the colloid is made of metallic nanostructures, such as silver and gold, resonant optical effects play a vital role, and the interaction leads to complex dynamics and assembly. This brief review aims to discuss some recent work on trapping plasmonic colloids with optical vortices and their lattices. The role of optical scattering and absorption has important implications on the underlying forces and torques, which is specifically enunciated. The effect of spin and orbital angular momentum in an optical vortex can lead to spin-orbit coupling dynamics, and these effects are highlighted with examples from the literature. In addition to assembly and dynamics, enhanced Brownian motion of plasmonic colloids under the influence of a vortex-lattice is discussed. The pedagogical aspects to understand the interaction between optical vortex and plasmonic colloids is emphasized.

I welcome comments on the review.

arxiv : https://arxiv.org/abs/2211.03547

New paper :”Optothermal evolution of active colloidal matter in defocused laser trap”

We have a new paper to be published in ACS Photonics on “Optothermal evolution of active colloidal matter in defocused laser trap”

In the context of non-equilibrium statistical mechanics, it is relevant to ask : how does a system of (active) Brownian particles respond to environmental cues ?

Structured light in the form of an optical trap can facilitate a platform to create unconventional, environmental cues in which Brownian particles can dynamically assemble and evolve as a function of space and time.

In this work, we utilize a simple defocused laser trap and study the evolutionary dynamics of thermally active colloids (polystyrene spheres infused with iron oxide). We observe a variety of (nonlinear) dynamical states including hovering of a pair, a kind of synchrony among the assembled colloids in the trap (see video).

Thanks to the great efforts of Dipta and Rahul from my group, we have been able to study and unveil the complex forces at play. The dual contribution of optical potential of the laser and thermophoretic interaction of colloids were revealed by systematic experiments and numerical simulations leading to this elaborate report.

This study further motivates interesting questions in the context of microscopic heat engines where the light and heat created in an optical trap can lead to some interesting nonlinear dynamics of soft matter systems. Another prospect is to characterize structured optothermal fields using Brownian motors as microscopic probes in an optical trap. More on this in the coming month….

all videos related to the work on our lab youtube channel

preprint version of the paper on arxiv : https://arxiv.org/abs/2203.08904

I will post the published version of the article when available

Roadmap for optical tweezers is on arxiv

I am delighted to share the arxiv link to Roadmap For Optical Tweezers : https://arxiv.org/abs/2206.13789

This document brings together researchers from 52 different affiliations across the globe to look into the accomplishments and future directions of optical tweezers.

My contribution towards roadmap appears on page 136, topic number 31 on — Raman scattering in (thermo)plasmonic tweezers.

In there, I discuss how plasmonic platforms can be used to generate attractive optothermal forces to trap and interrogate molecules and nanoparticles, down to single copy limit. I also discuss the challenges and opportunities of such a process.

Optical tweezers is one of the most powerful optical tools that finds utility not only in fundamental physics, but also in diverse applications including biology and medicine.

Ever since the Nobel prize-winning work of Arthur Ashkin, optical tweezers have evolved and continues to evolve into various forms. This roadmap article aims to capture this evolution, and to discuss the emerging capabilities and challenges of optical tweezers.

A big thank you to

Giovanni Volpe
Onofrio M. Maragò
and Halina Rubinzstein-Dunlop

for their leadership in this field and for the herculean task of coordinating and editing this roadmap….

The roadmap has been submitted to Journal of Physics : Photonics (IOP)